@article{SessiSilkinNechaevetal.2015, author = {Sessi, Paolo and Silkin, Vyacheslav M. and Nechaev, Ilya A. and Bathon, Thomas and El-Kareh, Lydia and Chulkov, Evgueni V. and Echenique, Pedro M. and Bode, Matthias}, title = {Direct observation of many-body charge density oscillations in a two-dimensional electron gas}, series = {Nature Communications}, volume = {6}, journal = {Nature Communications}, number = {8691}, doi = {10.1038/ncomms9691}, url = {http://nbn-resolving.de/urn:nbn:de:bvb:20-opus-145246}, year = {2015}, abstract = {Quantum interference is a striking manifestation of one of the basic concepts of quantum mechanics: the particle-wave duality. A spectacular visualization of this effect is the standing wave pattern produced by elastic scattering of surface electrons around defects, which corresponds to a modulation of the electronic local density of states and can be imaged using a scanning tunnelling microscope. To date, quantum-interference measurements were mainly interpreted in terms of interfering electrons or holes of the underlying band-structure description. Here, by imaging energy-dependent standing-wave patterns at noble metal surfaces, we reveal, in addition to the conventional surface-state band, the existence of an 'anomalous' energy band with a well-defined dispersion. Its origin is explained by the presence of a satellite in the structure of the many-body spectral function, which is related to the acoustic surface plasmon. Visualizing the corresponding charge oscillations provides thus direct access to many-body interactions at the atomic scale.}, language = {en} } @article{FiedlerElKarehEremeevetal.2014, author = {Fiedler, Sebastian and El-Kareh, Lydia and Eremeev, Sergey V. and Tereshchenko, Oleg E. and Seibel, Christoph and Lutz, Peter and Kokh, Konstantin A. and Chulkov, Evgueni V. and Kuznetsova, Tatyana V. and Grebennikov, Vladimir I. and Bentmann, Hendrik and Bode, Matthias and Reinert, Friedrich}, title = {Defect and structural imperfection effects on the electronic properties of BiTeI surfaces}, series = {New Journal of Physics}, volume = {16}, journal = {New Journal of Physics}, number = {075013}, issn = {1367-2630}, doi = {10.1088/1367-2630/16/7/075013}, url = {http://nbn-resolving.de/urn:nbn:de:bvb:20-opus-119467}, year = {2014}, abstract = {The surface electronic structure of the narrow-gap seminconductor BiTeI exhibits a large Rashba-splitting which strongly depends on the surface termination. Here we report on a detailed investigation of the surface morphology and electronic properties of cleaved BiTeI single crystals by scanning tunneling microscopy, photoelectron spectroscopy (ARPES, XPS), electron diffraction (SPA-LEED) and density functional theory calculations. Our measurements confirm a previously reported coexistence of Te- and I-terminated surface areas originating from bulk stacking faults and find a characteristic length scale of ~100 nm for these areas. We show that the two terminations exhibit distinct types of atomic defects in the surface and subsurface layers. For electronic states resided on the I terminations we observe an energy shift depending on the time after cleavage. This aging effect is successfully mimicked by depositon of Cs adatoms found to accumulate on top of the I terminations. As shown theoretically on a microscopic scale, this preferential adsorbing behaviour results from considerably different energetics and surface diffusion lengths at the two terminations. Our investigations provide insight into the importance of structural imperfections as well as intrinsic and extrinsic defects on the electronic properties of BiTeI surfaces and their temporal stability.}, language = {en} } @article{MaassBentmannSeibeletal.2016, author = {Maaß, Henriette and Bentmann, Hendrik and Seibel, Christoph and Tusche, Christian and Eremeev, Sergey V. and Peixoto, Thiago R.F. and Tereshchenko, Oleg E. and Kokh, Konstantin A. and Chulkov, Evgueni V. and Kirschner, J{\"u}rgen and Reinert, Friedrich}, title = {Spin-texture inversion in the giant Rashba semiconductor BiTeI}, series = {Nature Communications}, volume = {7}, journal = {Nature Communications}, doi = {10.1038/ncomms11621}, url = {http://nbn-resolving.de/urn:nbn:de:bvb:20-opus-173769}, year = {2016}, abstract = {Semiconductors with strong spin-orbit interaction as the underlying mechanism for the generation of spin-polarized electrons are showing potential for applications in spintronic devices. Unveiling the full spin texture in momentum space for such materials and its relation to the microscopic structure of the electronic wave functions is experimentally challenging and yet essential for exploiting spin-orbit effects for spin manipulation. Here we employ a state-of-the-art photoelectron momentum microscope with a multichannel spin filter to directly image the spin texture of the layered polar semiconductor BiTeI within the full two-dimensional momentum plane. Our experimental results, supported by relativistic ab initio calculations, demonstrate that the valence and conduction band electrons in BiTeI have spin textures of opposite chirality and of pronounced orbital dependence beyond the standard Rashba model, the latter giving rise to strong optical selection-rule effects on the photoelectron spin polarization. These observations open avenues for spin-texture manipulation by atomic-layer and charge carrier control in polar semiconductors.}, language = {en} }