@phdthesis{Weissenseel2022, author = {Weißenseel, Sebastian G{\"u}nter}, title = {Spin-Spin Interactions and their Impact on Organic Light-Emitting Devices}, doi = {10.25972/OPUS-25745}, url = {http://nbn-resolving.de/urn:nbn:de:bvb:20-opus-257458}, school = {Universit{\"a}t W{\"u}rzburg}, year = {2022}, abstract = {This work investigates the correlations between spin states and the light emission properties of organic light-emitting diodes (OLEDs), which are based on the principle of thermally activated delayed fluorescence. The spin-spin interactions responsible for this mechanism are investigated in this work using methods based on spin-sensitive electron paramagnetic resonance (EPR). In particular, this method has been applied to electrically driven OLEDs. The magnetic resonance has been detected by electroluminescence, giving this method its name: electroluminescence detected magnetic resonance (ELDMR). Initial investigations on a novel deep blue TADF emitter were performed. Furthermore, the ELDMR method was used in this work to directly detect the spin states in the OLED. These measurements were further underlined by time-resolved experiments such as transient electro- and photoluminescence.}, subject = {Elektronenspinresonanz}, language = {en} }