TY  - JOUR
A1  - Rewitz, Christian
A1  - Keitzl, Thomas
A1  - Tuchscherer, Philip
A1  - Goetz, Sebastian
A1  - Geisler, Peter
A1  - Razinskas, Gary
A1  - Hecht, Bert
A1  - Brixner, Tobias
T1  - Spectral-interference microscopy for characterization of functional plasmonic elements
JF  - Optics Express
N2  - Plasmonic modes supported by noble-metal nanostructures offer strong subwavelength electric-field confinement and promise the realization of nanometer-scale integrated optical circuits with well-defined functionality. In order to measure the spectral and spatial response functions of such plasmonic elements, we combine a confocal microscope setup with spectral interferometry detection. The setup, data acquisition, and data evaluation are discussed in detail by means of exemplary experiments involving propagating plasmons transmitted through silver nanowires. By considering and experimentally calibrating any setup-inherent signal delay with an accuracy of 1 fs, we are able to extract correct timing information of propagating plasmons. The method can be applied, e.g., to determine the dispersion and group velocity of propagating plasmons in nanostructures, and can be extended towards the investigation of nonlinear phenomena.
Y1  - 2012
U6  - http://nbn-resolving.de/urn/resolver.pl?urn:nbn:de:bvb:20-opus-85922
UR  - http://www.opticsinfobase.org/oe/fulltext.cfm?uri=oe-20-13-14632&id=238393
ER  - 
TY  - JOUR
A1  - Steinbacher, Andreas
A1  - Buback, Johannes
A1  - Nürnberger, Patrick
A1  - Brixner, Tobias
T1  - Precise and rapid detection of optical activity for accumulative femtosecond spectroscopy
JF  - Optics Express
N2  - We present polarimetry, i.e. the detection of optical rotation of light polarization, in a configuration suitable for femtosecond spectroscopy. The polarimeter is based on common-path optical heterodyne interferometry and provides fast and highly sensitive detection of rotatory power. Femtosecond pump and polarimeter probe beams are integrated into a recently developed accumulative technique that further enhances sensitivity with respect to single-pulse methods. The high speed of the polarimeter affords optical rotation detection during the pump-pulse illumination period of a few seconds. We illustrate the concept on the photodissociation of the enantiomers of methyl p-tolyl sulfoxide. The sensitivity of rotatory detection, i.e. the minimum rotation angle that can be measured, is determined experimentally including all noise sources to be 0.10 milli-degrees for a measurement time of only one second and an interaction length of 250 μm. The suitability of the presented setup for femtosecond studies is demonstrated in a non-resonant two-photon photodissociation experiment.
Y1  - 2012
U6  - http://nbn-resolving.de/urn/resolver.pl?urn:nbn:de:bvb:20-opus-85913
UR  - http://www.opticsinfobase.org/oe/fulltext.cfm?uri=oe-20-11-11838&id=233249
ER  - 
TY  - JOUR
A1  - Aeschlimann, Martin
A1  - Bauer, Michael
A1  - Bayer, Daniela
A1  - Brixner, Tobias
A1  - Cunovic, Stefan
A1  - Fischer, Alexander
A1  - Melchior, Pascal
A1  - Pfeiffer, Walter
A1  - Rohmer, Martin
A1  - Schneider, Christian
A1  - Strüber, Christian
A1  - Tuchscherer, Philip
A1  - Voronine, Dimitri V.
T1  - Optimal open-loop near-field control of plasmonic nanostructures
N2  - Optimal open-loop control, i.e. the application of an analytically derived control rule, is demonstrated for nanooptical excitations using polarization-shaped laser pulses. Optimal spatial near-field localization in gold nanoprisms and excitation switching is realized by applying a shift to the relative phase of the two polarization components. The achieved near-field switching confirms theoretical predictions, proves the applicability of predefined control rules in nanooptical light–matter interaction and reveals local mode interference to be an important control mechanism.
KW  - Chemie
Y1  - 2012
U6  - http://nbn-resolving.de/urn/resolver.pl?urn:nbn:de:bvb:20-opus-75256
ER  -