TY  - JOUR
A1  - Sessi, Paolo
A1  - Silkin, Vyacheslav M.
A1  - Nechaev, Ilya A.
A1  - Bathon, Thomas
A1  - El-Kareh, Lydia
A1  - Chulkov, Evgueni V.
A1  - Echenique, Pedro M.
A1  - Bode, Matthias
T1  - Direct observation of many-body charge density oscillations in a two-dimensional electron gas
JF  - Nature Communications
N2  - Quantum interference is a striking manifestation of one of the basic concepts of quantum mechanics: the particle-wave duality. A spectacular visualization of this effect is the standing wave pattern produced by elastic scattering of surface electrons around defects, which corresponds to a modulation of the electronic local density of states and can be imaged using a scanning tunnelling microscope. To date, quantum-interference measurements were mainly interpreted in terms of interfering electrons or holes of the underlying band-structure description. Here, by imaging energy-dependent standing-wave patterns at noble metal surfaces, we reveal, in addition to the conventional surface-state band, the existence of an 'anomalous' energy band with a well-defined dispersion. Its origin is explained by the presence of a satellite in the structure of the many-body spectral function, which is related to the acoustic surface plasmon. Visualizing the corresponding charge oscillations provides thus direct access to many-body interactions at the atomic scale.
KW  - scanning tunneling spectroscopy
KW  - acoustic surface plasmon
KW  - metal surfaces
KW  - Cu(111)
KW  - excitations
KW  - microscopy
KW  - local density
KW  - standing wave formation
KW  - states
KW  - steps
Y1  - 2015
U6  - http://nbn-resolving.de/urn/resolver.pl?urn:nbn:de:bvb:20-opus-145246
VL  - 6
IS  - 8691
ER  - 
TY  - JOUR
A1  - Christ, Andreas
A1  - Härtl, Patrick
A1  - Kloster, Patrick
A1  - Bode, Matthias
A1  - Leisegang, Markus
T1  - Influence of band structure on ballistic transport revealed by molecular nanoprobe
JF  - Physical Review Research
N2  - In this study we characterize the tautomerization of HPc on Cu(111) as a charge-carrier-induced reversible one-electron process. An analysis of the bias-dependent tautomerization rate finds an energy threshold that corresponds to the energy of the N-H stretching mode. By using the tautomerization of the molecule as a detector for charge carrier transport in the so-called molecular nanoprobe (MONA) technique, we provide evidence for an inhomogeneous coupling between the fourfold-symmetric molecule and sixfold-symmetric surface. We conclude the study by comparing the energy dependence of charge carrier transport on the Cu(111) to the Ag(111) surface. While the MONA technique is limited to the detection of hot-electron transport for Ag(111), our data reveal that the lower onset energy of the Cu surface state also allows for the detection of hot-hole transport. The influence of surface and bulk transport on the MONA technique is discussed.
KW  - tautomerization
KW  - HPc
KW  - Cu(111)
Y1  - 2022
U6  - http://nbn-resolving.de/urn/resolver.pl?urn:nbn:de:bvb:20-opus-300855
VL  - 4
IS  - 4
ER  -